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Reactions of garnet-based solid-state lithium electrolytes with water - A depth-resolved study
作者 :  Uhlenbruck, Sven; Dellen, Christian; Moeller, Soeren; Lobe, Sandra; Tsai, Chih-Long; Finsterbusch, Martin; Bram, Martin; Guillon, Olivier
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Garnet Li6.4La3Zr1.6Ta0.4O12 thin films prepared by magnetron sputtering were analysed by secondary ion mass spectrometry, nuclear reaction analysis and Rutherford backscattering to identify, localize and quantify the reactions associated with the presence of low amounts of water and carbon dioxide. Samples in a pristine state and after storage in an Argon-filled glove box for months were compared. Both, lithium hydroxide and lithium carbonate were detected, with carbon-containing species and hydrogen-containing having surprisingly different depth profiles.

关 键 词 :  Battery; Thin film; Secondary ion mass spectrometry; Nuclear reaction analysis; Raman microscopy
论文来源 :  SOLID STATE IONICS.2018,320:259-265
语种 :  英文
所属领域 :  >>> 海洋科学研究
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入库时间 :  2019-10-14
浏览次数 :  1